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Energy Transfer in Aqueous Light Harvesting Antennae Based on Brush-like Inter-Conjugated Polyelectrolyte Complexes.
Publication Type: Academic Journal
Source(s): Macromolecules [Macromolecules] 2022 Dec 13; Vol. 55 (23), pp. 10302-10311. Date of Electronic Publication: 2022 Nov 29.
Abstract: Conjugated polyelectrolytes (CPEs) have the potential to serve as building blocks of artificial light-harvesting systems. This is primarily due to their delocalized electronic states and potential for hierarchical self-assembly. We showed previously th...
Two-Dimensional Porphyrin-Based Covalent Organic Framework with Enlarged Inter-layer Spacing for Tunable Photocatalytic CO 2 Reduction.
Publication Type: Academic Journal
Source(s): ACS applied materials & interfaces [ACS Appl Mater Interfaces] 2022 Sep 14; Vol. 14 (36), pp. 41122-41130. Date of Electronic Publication: 2022 Aug 31.
Abstract: Two-dimensional (2D) porphyrin-based covalent organic frameworks (COFs) are one of the most promising candidates for photocatalytic carbon dioxide reduction reaction (CO 2 RR), which however still suffer from the hindered mass transfer during the catal...
Ambiphilic Behavior of Ge(II)-Pseudohalides in Inter- and Intramolecular Frustrated Lewis Pair Alkyne Addition Reactions.
Publication Type: Academic Journal
Source(s): Inorganic chemistry [Inorg Chem] 2022 Nov 21; Vol. 61 (46), pp. 18670-18677. Date of Electronic Publication: 2022 Nov 08.
Abstract: The reaction of the germylene chloride (NacNac)GeCl ( 1 , NacNac = CH{(CMe)(2,6- i Pr 2 C 6 H 3 N)} 2 ), phenylacetylene, and B(C 6 F 5 ) 3 gives the intermolecular frustrated Lewis pair (FLP) addition product 2 . In this case, the...
Inter-Electronic Interaction between Ni and Mo in Electrodeposited Ni-Mo-P on 3D Copper Foam Enables Hydrogen Evolution Reaction at Low Overpotential.
Publication Type: Academic Journal
Source(s): Inorganic chemistry [Inorg Chem] 2022 Nov 14; Vol. 61 (45), pp. 18253-18259. Date of Electronic Publication: 2022 Oct 30.
Abstract: Electrocatalytic hydrogen evolution reaction (HER) via water electrolysis has been considered the most effective and sustainable route to produce clean hydrogen. Designing and structure optimization are the two important parameters to develop an afford...
Role of Half-of-Sites Reactivity and Inter-Subunit Communications in DAHP Synthase Catalysis and Regulation.
Publication Type: Academic Journal
Source(s): Biochemistry [Biochemistry] 2022 Oct 18; Vol. 61 (20), pp. 2229-2240. Date of Electronic Publication: 2022 Oct 05.
Abstract: α-Carboxyketose synthases, including 3-deoxy-d- arabino heptulosonate 7-phosphate synthase (DAHPS), are long-standing targets for inhibition. They are challenging targets to create tight-binding inhibitors against, and inhibitors often display half-of-...
Intra- and Inter-Self-Assembly of Identical Supramolecules on Silver Surfaces.
Publication Type: Academic Journal
Source(s): The journal of physical chemistry letters [J Phys Chem Lett] 2022 Sep 29; Vol. 13 (38), pp. 8902-8907. Date of Electronic Publication: 2022 Sep 20.
Abstract: Self-assembly of identical organometallic supramolecules into ordered superstructures is of great interest in both chemical science and nanotechnology due to its potential to generate neoteric properties through collective effects. In this work, we dem...
Inter- and Intraindividual Differences in the Capacity of the Human Intestinal Microbiome in Fecal Slurries to Metabolize Fructoselysine and Carboxymethyllysine.
Publication Type: Academic Journal
Source(s): Journal of agricultural and food chemistry [J Agric Food Chem] 2022 Sep 21; Vol. 70 (37), pp. 11759-11768. Date of Electronic Publication: 2022 Sep 07.
Abstract: The advanced glycation endproduct carboxymethyllysine and its precursor fructoselysine are present in heated, processed food products and are considered potentially hazardous for human health. Upon dietary exposure, they can be degraded by human coloni...
Injectable Hydrogels Based on Inter-Polyelectrolyte Interactions between Hyaluronic Acid, Gelatin, and Cationic Cellulose Nanocrystals.
Publication Type: Academic Journal
Source(s): Biomacromolecules [Biomacromolecules] 2022 Aug 08; Vol. 23 (8), pp. 3222-3234. Date of Electronic Publication: 2022 Jun 30.
Abstract: The present work dealt with the development of physically cross-linked injectable hydrogels with potential applications in tissue engineering. The hydrogels were composed of a ternary mixture of a polyanion and a polyampholyte, hyaluronic acid (HA) and...
Solution-State Inter-Copper Distribution of Redox Partner-Linked Copper Nitrite Reductases: A Pulsed Electron-Electron Double Resonance Spectroscopy Study.
Publication Type: Academic Journal
Source(s): The journal of physical chemistry letters [J Phys Chem Lett] 2022 Aug 04; Vol. 13 (30), pp. 6927-6934. Date of Electronic Publication: 2022 Jul 22.
Abstract: Copper nitrite reductases (CuNiRs) catalyze the reduction of nitrite to form nitric oxide. In recent years, new classes of redox partner linked CuNiRs have been isolated and characterized by crystallographic techniques. Solution-state biophysical studi...
Effect of In Vitro Solvation Conditions on Inter- and Intramolecular Assembly of Full-Length TDP-43.
Publication Type: Academic Journal
Source(s): The journal of physical chemistry. B [J Phys Chem B] 2022 Jul 07; Vol. 126 (26), pp. 4799-4813. Date of Electronic Publication: 2022 Jun 25.
Abstract: Cellular stress is a major cause of neurodegenerative diseases. In particular, in amyotrophic lateral sclerosis (ALS), around 90% of the cases are believed to occur due to aggregation and misfolding of TDP-43 protein in neurons due to aging and chronic...