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Inter- and Intraindividual Differences in the Capacity of the Human Intestinal Microbiome in Fecal Slurries to Metabolize Fructoselysine and Carboxymethyllysine.
Publication Type: Academic Journal
Source(s): Journal of agricultural and food chemistry [J Agric Food Chem] 2022 Sep 21; Vol. 70 (37), pp. 11759-11768. Date of Electronic Publication: 2022 Sep 07.
Abstract: The advanced glycation endproduct carboxymethyllysine and its precursor fructoselysine are present in heated, processed food products and are considered potentially hazardous for human health. Upon dietary exposure, they can be degraded by human coloni...
Two-Dimensional Porphyrin-Based Covalent Organic Framework with Enlarged Inter-layer Spacing for Tunable Photocatalytic CO 2 Reduction.
Publication Type: Academic Journal
Source(s): ACS applied materials & interfaces [ACS Appl Mater Interfaces] 2022 Sep 14; Vol. 14 (36), pp. 41122-41130. Date of Electronic Publication: 2022 Aug 31.
Abstract: Two-dimensional (2D) porphyrin-based covalent organic frameworks (COFs) are one of the most promising candidates for photocatalytic carbon dioxide reduction reaction (CO 2 RR), which however still suffer from the hindered mass transfer during the catal...
Injectable Hydrogels Based on Inter-Polyelectrolyte Interactions between Hyaluronic Acid, Gelatin, and Cationic Cellulose Nanocrystals.
Publication Type: Academic Journal
Source(s): Biomacromolecules [Biomacromolecules] 2022 Aug 08; Vol. 23 (8), pp. 3222-3234. Date of Electronic Publication: 2022 Jun 30.
Abstract: The present work dealt with the development of physically cross-linked injectable hydrogels with potential applications in tissue engineering. The hydrogels were composed of a ternary mixture of a polyanion and a polyampholyte, hyaluronic acid (HA) and...
Solution-State Inter-Copper Distribution of Redox Partner-Linked Copper Nitrite Reductases: A Pulsed Electron-Electron Double Resonance Spectroscopy Study.
Publication Type: Academic Journal
Source(s): The journal of physical chemistry letters [J Phys Chem Lett] 2022 Aug 04; Vol. 13 (30), pp. 6927-6934. Date of Electronic Publication: 2022 Jul 22.
Abstract: Copper nitrite reductases (CuNiRs) catalyze the reduction of nitrite to form nitric oxide. In recent years, new classes of redox partner linked CuNiRs have been isolated and characterized by crystallographic techniques. Solution-state biophysical studi...
Effect of In Vitro Solvation Conditions on Inter- and Intramolecular Assembly of Full-Length TDP-43.
Publication Type: Academic Journal
Source(s): The journal of physical chemistry. B [J Phys Chem B] 2022 Jul 07; Vol. 126 (26), pp. 4799-4813. Date of Electronic Publication: 2022 Jun 25.
Abstract: Cellular stress is a major cause of neurodegenerative diseases. In particular, in amyotrophic lateral sclerosis (ALS), around 90% of the cases are believed to occur due to aggregation and misfolding of TDP-43 protein in neurons due to aging and chronic...
Decoding Key Transient Inter-Catalyst Interactions in a Reductive Metallaphotoredox-Catalyzed Allylation Reaction.
Publication Type: Academic Journal
Source(s): Journal of the American Chemical Society [J Am Chem Soc] 2022 Jun 22; Vol. 144 (24), pp. 10912-10920. Date of Electronic Publication: 2022 Jun 08.
Abstract: Metallaphotoredox chemistry has recently witnessed a surge in interest within the field of synthetic organic chemistry through the use of abundant first-row transition metals combined with suitable photocatalysts. The intricate details arising from the...
Enantioselective Inter- and Intramolecular Sulfenofunctionalization of Unactivated Cyclic and ( Z )-Alkenes.
Publication Type: Academic Journal
Source(s): ACS catalysis [ACS Catal] 2022 Jun 17; Vol. 12 (12), pp. 7377-7385. Date of Electronic Publication: 2022 Jun 07.
Abstract: A method for the enantioselective, Lewis base-catalyzed sulfenofunctionalization of cyclic and ( Z )-alkenes is reported. The intermediate thiiranium ion generated in the presence of a selenophosphoramide catalyst is intercepted by a variety of nucleop...
Inter-Leaflet Phospholipid Exchange Impacts the Ligand Density Available for Protein Binding at Supported Lipid Bilayers.
Publication Type: Academic Journal
Source(s): Langmuir : the ACS journal of surfaces and colloids [Langmuir] 2022 Jun 07; Vol. 38 (22), pp. 6967-6976. Date of Electronic Publication: 2022 May 26.
Abstract: Phospholipid bilayers formed at solid-liquid interfaces have garnered interest as mimics of cell membranes to model association reactions of proteins with lipid bilayer-tethered ligands. Despite the importance of understanding how ligand density in a l...
Synergizing Inter and Intraband Transitions in Defective Tungsten Oxide for Efficient Photocatalytic Alcohol Dehydration to Alkenes.
Publication Type: Academic Journal
Source(s): JACS Au [JACS Au] 2022 May 13; Vol. 2 (5), pp. 1160-1168. Date of Electronic Publication: 2022 May 13 (Print Publication: 2022).
Abstract: Photocatalysis under mild conditions is an intriguing avenue for organic chemical manufacturing to confront the serious fossil energy crisis. Herein, we report a direct light-driven alkene production through alcohol dehydration, using nonstoichiometric...
Accelerating Protein Folding Molecular Dynamics Using Inter-Residue Distances from Machine Learning Servers.
Publication Type: Academic Journal
Source(s): Journal of chemical theory and computation [J Chem Theory Comput] 2022 Mar 08; Vol. 18 (3), pp. 1929-1935. Date of Electronic Publication: 2022 Feb 08.
Abstract: Recently, predicting the native structures of proteins has become possible using computational molecular physics (CMP)─physics-based force fields sampled with proper statistics─but only for small proteins. Algorithms with better scaling are needed. We ...